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nonequilibrium interface motion

Nonequilibrium interface behavior in Cahn-Hilliard models for Li-ion batteries

Experiments, numerical simulations, and analytical calculations are used to calibrate a diffuse-interface Cahn-Hilliard model of Li-Sn thin film electrodes that experience a transformation from Sn to Li2Sn5. It is shown that a concentration-gradient dependent mobility can be used in the Cahn-Hilliard equation to give the interface a finite mobility and capture its nonequilibrium behavior.

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